The original members were Joe Grier (lead), Steve Brown (first tenor), Glenmore Jackson (second tenor), Leroy Binns (baritone), and Ross Buford (bass). Initially called "The Thrilltones," they changed their name at the suggestion of their manager, Les Cooper.

Their most famous song, "Deserie," was released in 1957 on Danny Robinson's undefined label. Although it didn’t chart nationally, it became popular in New York and is considered a Doo-Wop classic. The success of "Deserie" led to performances at prestigious venues like the Apollo Theater in Harlem and the Regal Theater in Chicago. In 1967 they broke up.

Despite their talent and regional popularity, The Charts were unable to achieve broader commercial success. However, their contribution to the Doo-Wop genre, especially with "Deserie," remains a significant part of music history.